Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Adhésion métal–polymère : des simulations atomiques révèlent les mécanismes d’accrochage à l’interface
Des chercheurs de l’Osaka Metropolitan University ont élucidé les interactions moléculaires qui gouvernent l’adhésion directe entre polymères et métaux, ouvrant la voie à de nouveaux matériaux hybrides légers pour les transports. Grâce à des simulations de dynamique moléculaire tout-atome, ils ont étudié la liaison entre des polyamides (PA6 et PAMXD6) et une surface d’alumine présentant ou non des groupements hydroxyles. Les modèles ont permis d’observer en temps réel l’organisation des chaînes polymères à l’interface : segments adsorbés (trains), boucles libres et extrémités (tails). Avant la déformation irréversible du système (régime élastique), la résistance à la traction dépend principalement de la chimie du polymère, l’aromatique PAMXD6 se montrant plus rigide que le PA6. Après le seuil de plasticité, c’est la chimie de surface du métal qui devient déterminante : sur une alumine hydroxylée, le PAMXD6 se désorbe tandis que le PA6 se réorganise sans rupture complète, transformant ses boucles en chaînes tendues. Sur une surface non hydroxylée, les deux polymères conservent une forte cohésion via des segments adsorbés stables. Ces observations atomistiques expliquent pourquoi certaines combinaisons métal–plastique résistent mieux que d’autres et fournissent un cadre rationnel pour optimiser les traitements de surface et la conception moléculaire des polymères d’adhésion, favorisant le développement de structures hybrides plus durables et énergétiquement efficientes.
https://phys.org/news/2025-11-plastics-metals-atomic-scale-molecular.html
Une voie inédite pour rendre les polyméthacrylates dégradables grâce à une copolymérisation radicalaire assistée par modélisation
Des chercheurs français et belges ont réussi à surmonter une limite jugée jusqu’ici « impossible » en chimie des polymères : introduire des liaisons dégradables dans les polyméthacrylates industriels comme le PMMA. Publiée dans Nature Communications, leur étude démontre qu’il est possible d’insérer des unités thionolactones – porteuses de liaisons thioesters clivables – au sein de chaînes polyméthacrylates grâce à un troisième comonomère « auxiliaire » (acrylate ou maléimide). Cette approche de copolymérisation radicalaire à ouverture de cycle (rROP) permet de créer des triades structurales contrôlées (par ex. PhMal–DOT–PhMal) assurant la dégradabilité sans altérer les propriétés mécaniques du polymère. Appuyée par des simulations Monte Carlo couplées (CMMC), la stratégie optimise les conditions de synthèse pour obtenir des polymères de haut poids moléculaire capables, après dégradation, de se fragmenter jusqu’à vingt-cinq fois en oligomères. Les chercheurs démontrent aussi la robustesse du procédé pour d’autres méthacrylates, dont des polymères hydrosolubles à potentiel biomédical, dégradables en milieu aqueux. Cette avancée associe conception computationnelle et chimie radicalaire pour introduire, de manière précise, des liaisons faibles dans des polymères auparavant non recyclables. Elle ouvre la voie à une nouvelle génération de matériaux méthacrylates à dégradation programmable, conciliant performance industrielle et fin de vie maîtrisée, et redéfinit les perspectives de durabilité pour l’une des familles plastiques les plus répandues au monde.
Nature Le recyclage du plastique, une réalité industrielle appuyée par la science
La campagne “Recycling is Real” de la Plastics Industry Association met en lumière les avancées concrètes du recyclage des plastiques à travers les États-Unis, en s’appuyant sur des technologies de pointe comme la thermoformage de plastiques post-consommation. En filmant des sites comme celui de Plastic Ingenuity dans le Wisconsin, qui transforme les déchets plastiques en emballages pour les secteurs alimentaire et médical, l’initiative démontre comment des approches industrielles fondées sur la science des matériaux et l’ingénierie environnementale permettent de réintégrer le plastique dans une boucle circulaire. Cette démonstration pragmatique de recyclage vise aussi à corriger les idées reçues en soulignant que l’innovation technique et la rigueur scientifique sont au cœur des solutions pour réduire l’impact environnemental du plastique.
https://www.plasticstoday.com/sustainability/plastics-showcases-real-recycling-success-stories
Recycler le PVC sans risque, c’est (enfin) possible
Le PVC est un plastique omniprésent… et l’un des plus difficiles à recycler. Trop chloré, il résiste aux procédés classiques et génère des sous-produits toxiques lorsqu’on tente de le brûler ou de le dégrader. Une équipe chinoise a mis au point une solution élégante et propre : un catalyseur sur-mesure (LaFe₀.₃Al₀.₇O₃) qui déclenche une « cascade » de réactions douces dans l’eau, à température ambiante.
Ce procédé active d’abord une forme spéciale d’oxygène singulet pour retirer les atomes de chlore de manière sélective. Ensuite, des radicaux hydroxyles attaquent la chaîne carbonée, menant à une dépolymérisation complète. Résultat : le PVC est transformé en CO₂ et en hydrocarbures liquides réutilisables, sans aucun résidu solide ni composé chloré toxique.
Une analyse du cycle de vie montre que cette approche réduit drastiquement les émissions et les impacts environnementaux par rapport à l’enfouissement ou à l’incinération. C’est un bel exemple de chimie durable, qui transforme un plastique problématique en ressource utile — et ouvre la voie à un recyclage plus propre et plus circulaire.
Nature Nanofiltration membranaire : une percée pour purifier et recycler les plastiques sans les dégrader
Des chercheurs canadiens proposent une approche inédite de recyclage physique des plastiques fondée sur la nanofiltration membranaire. Publiée dans Communications Chemistry, l’étude démontre qu’il est possible d’éliminer efficacement les additifs et les fragments de polymères dégradés en exploitant un simple principe de séparation par taille moléculaire. Les polymères, dont les masses molaires dépassent 100 000 g/mol, sont des macromolécules bien plus volumineuses que les additifs (200–2000 g/mol). En dissolvant le plastique dans un solvant sélectif puis en le soumettant à une membrane céramique à pores nanométriques, les petites molécules migrent vers le perméat tandis que les chaînes polymères restent dans le rétentat. Appliqué au polystyrène contaminé par l’hexabromocyclododécane (HBCD), un retardateur de flamme interdit, le procédé atteint plus de 90 % d’élimination des contaminants tout en supprimant les chaînes courtes oxydées, améliorant ainsi la qualité du polymère recyclé. Ce système, pilotable par simple ajustement du volume de solvant ou de la pression transmembranaire, permet de contrôler précisément la pureté finale du produit. Compatible avec les polyoléfines, PVC, polyuréthanes et polystyrènes — soit près de 70 % du marché mondial des plastiques —, cette technologie comble l’écart entre recyclage mécanique et recyclage chimique. Sa scalabilité industrielle et sa capacité à générer des résines « quasi vierges » ouvrent la voie à un recyclage circulaire haute valeur ajoutée, limitant les pertes de matière et la dépendance aux ressources fossiles.
Nature Polymérisation induite par vinyl-aza-[3]cumulène : une voie stéréocontrôlée vers des poly(sulfonylamidines) intelligents pour la délivrance de médicaments
Une équipe chinoise a mis au point une nouvelle réaction multicomposante cuivre-catalysée permettant d’accéder à des polymères inédits à base de poly(diényle-N-sulfonylamidines), via des intermédiaires réactifs jusque-là inconnus : les vinyl-aza-[3]cumulènes. Ces espèces hautement électrophiles, formées in situ à partir d’esters, d’amines et d’azotures, induisent une polymérisation régiosélective et stéréocontrôlée donnant exclusivement des motifs diéniques de configuration E. L’approche permet la synthèse de polymères bien définis, thermiquement stables et hydrolysables, dont la dégradation en milieu basique libère des diénamides structurés. Grâce à leur squelette conjugué et à la présence de groupes sulfonylamidine zwitterioniques, ces macromolécules s’auto-assemblent spontanément en nanoparticules chargées négativement en milieu aqueux, capables d’encapsuler la doxorubicine par interactions électrostatiques et hydrophobes. Ces nanoparticules présentent un comportement de libération contrôlé par le pH, libérant plus de 80 % du médicament à pH acide (5–6), ce qui les rend adaptées à la délivrance ciblée en environnement tumoral. L’étude démontre ainsi que la conception rationnelle d’intermédiaires cumulènes azotés ouvre un accès inédit à des polymères fonctionnels stéréodéfinis et stimuli-réactifs, combinant stabilité, dégradabilité et auto-organisation. Cette avancée relie chimie des cumulènes, polymérisation multicomposante et nanomédecine, élargissant le champ des matériaux polymères intelligents pour la vectorisation thérapeutique.
![Vinyl-aza-[3]cumulene intermediates induced polymerization for accessing E-dienyl poly(sulfonylamidines) towards pH-responsive drug delivery - Nature Communications](https://media.springernature.com/m685/springer-static/image/art%3A10.1038%2Fs41467-025-65320-y/MediaObjects/41467_2025_65320_Fig1_HTML.png)
Nature Lorem ipsum dolor sit amet, consectetur adipiscing elit. Sed posuere tincidunt quam sit amet viverra. Nam in consequat nulla. Nunc rhoncus orci vitae arcu sagittis, in auctor nibh posuere. Donec ut nulla id enim tempor feugiat.
Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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