Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Transformer le polystyrène en nylon : un recyclage hybride prometteur
Le polystyrène, omniprésent dans les emballages et objets du quotidien, reste un cauchemar écologique : difficile à recycler, il finit souvent incinéré ou enfoui. Une équipe de chercheurs vient de franchir une étape décisive en proposant une méthode hybride, à la croisée de la chimie et de la biotechnologie, pour le transformer en acide adipique – un ingrédient clé du nylon.
Le processus commence par une dépolymérisation chimique du polystyrène en acide benzoïque. Cette transformation s’appuie sur une réaction d’oxydation catalytique optimisée, rendue plus efficace grâce à un solvant innovant : l’acide benzoïque lui-même. Ce choix permet une dissolution homogène du plastique, facilitant sa conversion.
Deuxième étape : l’acide benzoïque est ensuite métabolisé par une bactérie génétiquement modifiée (Pseudomonas putida), qui le transforme en acide muconique. Enfin, une simple hydrogénation catalytique permet d’obtenir de l’acide adipique, composant essentiel du nylon 6,6.
Cette filière complète de recyclage transforme un plastique problématique en un produit à haute valeur ajoutée, avec des émissions de gaz à effet de serre considérablement réduites par rapport à la voie pétrochimique classique. Elle ouvre des perspectives concrètes pour une économie circulaire des plastiques, en combinant innovations catalytiques et savoir-faire biologique.
Nature
PolyMetriX : un écosystème open source pour standardiser la chimie numérique des polymères
PolyMetriX propose une bibliothèque Python unifiée qui couvre l’ensemble du flux de travail en chimie des polymères assistée par données, de l’accès aux jeux de données jusqu’à l’entraînement et l’évaluation des modèles. L’innovation clé réside dans une featurisation hiérarchique qui extrait des descripteurs au niveau du polymère complet, de l’ossature et des chaînes latérales, surmontant les limites des empreintes de type Morgan et améliorant la robustesse en extrapolation. La plateforme s’appuie sur un jeu de référence Tg et introduit des stratégies de découpe des données adaptées aux polymères (LOCOCV, splits fondés sur la propriété) qui testent la généralisation dans des scénarios proches de la découverte de matériaux. Conçue avec une API modulaire inspirée de matminer/scikit-learn, elle harmonise l’ingestion de données, la représentation chimique (RDKit, PSMILES) et l’intégration modèle, tout en prenant en charge des systèmes multi-composants (mélanges polymère-molécule) via des comparateurs de descripteurs cohérents. Les résultats indiquent des performances prédictives supérieures et plus stables que les approches usuelles, avec des vecteurs de caractéristiques plus compacts et interprétables. Au-delà de la recherche académique, l’écosystème offre des repères reproductibles pour l’évaluation industrielle (formulation, mise à l’échelle, criblage virtuel) et jette les bases d’une normalisation des pratiques en polymère-informatique. En articulant design de descripteurs, curation de données et protocoles d’évaluation réalistes, PolyMetriX établit un socle communautaire pour accélérer la découverte assistée par IA de polymères à propriétés maîtrisées.
Nature Production catalytique de lactones biosourcées
La transition vers une économie circulaire des plastiques repose sur le développement de monomères renouvelables capables de donner naissance à des polymères recyclables chimiquement. Dans une revue publiée dans Nature Reviews Chemistry, Gregg Beckham et ses collaborateurs synthétisent les avancées récentes sur la production de lactones biosourcées, briques moléculaires essentielles pour la conception de polyesters circulaires. Les auteurs décrivent les voies catalytiques permettant de convertir des diols, des acides hydroxycarboxyliques et des acides dicarboxyliques issus de la biomasse en lactones, en insistant sur les critères de rendement atomique, d’efficacité énergétique et de scalabilité industrielle. L’analyse thermodynamique des processus guide le choix des conditions opératoires — type de réacteur, phase réactionnelle, rôle des solvants — afin d’optimiser la conversion tout en minimisant les déchets. Deux approches sont distinguées : la conversion directe de substrats biologiques en lactones et les voies indirectes via des intermédiaires chimiques. La revue met également en lumière la complémentarité entre biocatalyse métabolique et chimie de transformation catalytique, montrant que de nombreux précurseurs de lactones peuvent être dérivés de sucres, d’acides gras ou d’intermédiaires de fermentation. En reliant design catalytique, modélisation énergétique et durabilité, cette synthèse établit les fondements scientifiques d’une production circulaire de monomères polymériques issue du carbone renouvelable, ouvrant la voie à une chimie des matériaux affranchie des ressources fossiles.
Nature Recycler le polyacrylonitrile
Une équipe de chercheurs européens propose une avancée majeure pour la valorisation chimique des polymères à base d’acrylonitrile, tels que le SAN et l’ABS, dont le recyclage restait jusqu’ici limité en raison du risque d’émission de gaz toxiques (HCN, NOx). Publiée dans Nature Communications, leur étude décrit un procédé catalytique innovant de “shuttle catalysis” au palladium permettant de transférer les unités cyanure (HCN) du polymère vers une molécule accepteur, sans libérer de gaz dangereux. Ce mécanisme transforme simultanément la chaîne polymère en un résidu carboné réutilisable et génère un composé nitrile exploitable comme brique chimique de synthèse. En ajustant les conditions, la méthode peut soit produire des nitriles avec des rendements quasi quantitatifs, soit déshydrocyanater complètement les polymères en utilisant l’éthylène comme capteur de HCN, aboutissant à la formation de propionitrile, précurseur industriel régénérable en acrylonitrile. Les analyses spectroscopiques (NMR, FTIR) confirment la disparition des groupements nitriles au profit de doubles liaisons C=C, ouvrant la voie à l’upcycling du polymère défini : ethenolyse, pyrolyse sélective ou oxydation en acides aromatiques valorisables. Fait marquant, le procédé s’applique aussi à des déchets commerciaux, notamment les briques LEGO®, démontrant sa robustesse et son potentiel industriel. Cette approche modulaire illustre un nouveau paradigme de chimie circulaire, où les plastiques nitrilés deviennent des sources sûres et réactives d’azote et de carbone, conciliant sécurité, rendement et durabilité.
Nature Électrolyte polymère gélifié sans fluor pour batteries au lithium métal stables et durables
Des chercheurs ont mis au point un électrolyte polymère gélifié totalement dépourvu de fluor capable de stabiliser l’interface électrolytique solide (SEI) dans les batteries au lithium métal. Publiée dans Nature Communications, cette étude introduit un copolymère fluorine-free, nommé PVM-GPE, qui forme spontanément une SEI hybride riche en oxyde et nitrure de lithium (Li₂O/Li₃N). Cette couche inorganique assure une migration ionique rapide, une réduction des réactions parasites et une croissance homogène du lithium, empêchant ainsi la formation de dendrites. Le réseau polymère, obtenu par copolymérisation du carbonate de vinylène et du N,N’-méthylènebisacrylamide, combine liaisons hydrogène, ancrages anioniques et forte polarité, favorisant un transport sélectif et stable des ions Li⁺. Ce système, à la fois quasi-solide et hautement conducteur, permet d’atteindre une rétention de capacité de 84,7 % après 800 cycles à fort régime (3 C), surpassant les électrolytes fluorés conventionnels tout en éliminant leurs coûts et impacts environnementaux. L’analyse structurale révèle que la SEI favorise la croissance cristallographique du lithium le long du plan (200), plus stable et moins réactif, améliorant la durabilité des interfaces électrode-électrolyte. Compatible avec des cathodes riches en nickel (NCM811/NCM90), l’électrolyte maintient sa performance sous tension élevée (4,5 V) et dans des cellules poche de 1 Ah. En alliant conception moléculaire, chimie verte et ingénierie interfaciale, cette approche ouvre une voie durable vers des batteries solides-état performantes sans recours au fluor, conciliant sécurité, densité énergétique et circularité des matériaux.
Nature Recyclage éco-efficient du Téflon®
Une équipe de l’Université de Newcastle, en collaboration avec l’Université de Birmingham, a mis au point un procédé propre et économe en énergie permettant de décomposer le Téflon® (PTFE), polymère réputé pour son inertie chimique et thermique, en composés fluorés réutilisables. Publiée dans le Journal of the American Chemical Society, cette recherche démontre que l’application d’une énergie mécanique — par simple agitation dans un broyeur à billes — suffit, en présence de sodium métallique, à rompre les fortes liaisons carbone-fluor du polymère à température ambiante, sans solvants ni chauffage. Le Téflon® est ainsi converti en fluorure de sodium, matière première non toxique couramment utilisée en dentifrice et dans la synthèse de molécules pharmaceutiques. Grâce à une caractérisation fine par résonance magnétique nucléaire à l’état solide, les chercheurs confirment l’absence de sous-produits, validant l’efficacité et la pureté du recyclat. Ce procédé s’inscrit dans le cadre émergent de la mécan chimie verte, qui substitue l’énergie mécanique à la chaleur ou aux solvants pour initier des réactions propres. En offrant une voie circulaire pour récupérer le fluor à partir de déchets polymériques résistants, cette approche pourrait transformer la gestion des plastiques fluorés, traditionnellement sources de « polluants éternels », en une ressource chimique renouvelable. Elle marque une étape décisive vers une économie du fluor durable, conciliant innovation scientifique et responsabilité environnementale.
https://www.eurekalert.org/news-releases/1102562
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Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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Les partenaires
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hutchinson
http://www.hutchinson.com/fr
logo-ispa_coul_fond-fonce
http://www.ispa.asso.fr
LPMC
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http://www.waters.com
ICS
https://www-ics.u-strasbg.fr/
lrccp
http://www.ispa.asso.fr
cnrs
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arkema
http://www.coatex.com
Logo-ChemSuD
http://www.ispa.asso.fr
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