Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Accélération de la dégradation du poly(acide lactique) par insertion de liaisons thionoesters dans la chaîne principale
Cette recherche propose une stratégie novatrice pour améliorer la biodégradabilité du poly(acide lactique) en modifiant sa structure de chaîne principale par l’introduction de liaisons thionoesters, obtenues via la copolymérisation en ouverture de cycle du lactide avec son analogue thionocarbonylé. Cette approche moléculaire remplace partiellement les oxygènes carbonylés du PLA par des atomes de soufre, affaiblissant ainsi les liaisons ester tout en préservant les propriétés thermiques et mécaniques du polymère d’origine. Les copolymères obtenus conservent une stabilité élevée en milieu aqueux, mais présentent une dégradation sélective rapide sous stimulus chimique, notamment en présence d’amines, traduisant une rupture ciblée des liaisons thionoesters dans la chaîne. Cette dégradation contrôlée réduit efficacement la masse molaire et facilite la biodégradation ultérieure dans les environnements naturels. L’innovation de cette étude réside dans la mise au point d’une méthodologie de copolymérisation simple, adaptable et modulable permettant d’ajuster finement la proportion de sites labiles sans altérer la performance du matériau. En offrant une solution structurelle au problème de la persistance environnementale du PLA, cette stratégie ouvre la voie à une nouvelle génération de polyesters biosourcés à dégradation programmée, conciliant durabilité, stabilité fonctionnelle et circularité potentielle des plastiques à usage unique.
Nature Des tissus polymères fonctionnalisés à la défensine pour lutter contre les infections résistantes et accélérer la cicatrisation
Des chercheurs ont mis au point un pansement polymère antibactérien de nouvelle génération capable de neutraliser les bactéries multirésistantes, les biofilms et les toxines qui retardent la cicatrisation cutanée. Ce matériau innovant repose sur la conjugaison chimique d’une défensine humaine modifiée (HD5-myr), un peptide antimicrobien naturel, à des fibres de polyalcool vinylique (PVA) à l’aide d’un agent de couplage. Ce procédé industriel en une seule étape permet d’obtenir une toile non tissée bioactive dont la surface élimine les bactéries par contact direct, sans diffusion d’antibiotiques, tout en empêchant la formation de biofilms et la libération d’endotoxines. Le PVA@HD5-myr conserve la structure et l’activité biologique du peptide, agissant par désorganisation des membranes bactériennes et neutralisation des endotoxines issues des infections à Gram négatif. Testé sur des plaies infectées chez la souris, ce pansement a favorisé une cicatrisation plus rapide, une réduction nette de la charge bactérienne et une inflammation limitée, tout en affichant une biocompatibilité élevée. En combinant la résistance mécanique du polymère et la puissance antimicrobienne d’un peptide humain, cette approche inaugure une nouvelle génération de matériaux de soin intelligents, capables de prévenir les infections nosocomiales et de réduire le recours aux antibiotiques dans le traitement des plaies chroniques et résistantes.
Nature Polymères à base de cyclodextrine : un adsorbant ultra-rapide pour éliminer les PFAS de l’eau
Une équipe internationale a mis au point un nouveau polymère réticulé à base de β-cyclodextrine capable d’éliminer presque instantanément les substances per- et polyfluoroalkylées (PFAS), y compris leurs formes à chaîne courte réputées difficiles à piéger. Ce matériau innovant repose sur une architecture tripode aminée servant de réticulant, qui confère au réseau polymère une double affinité : inclusion hydrophobe des molécules fluorées dans les cavités de la cyclodextrine et interactions électrostatiques attractives entre les groupes amines protonés et les PFAS anioniques. Cette synergie permet d’atteindre une adsorption quasi complète en quelques minutes, surpassant largement les charbons activés et résines conventionnels, tout en maintenant son efficacité dans des eaux réelles riches en co-polluants. Le matériau conserve ses performances après plusieurs cycles d’adsorption-désorption, validant sa stabilité chimique et sa réutilisabilité. Ce travail illustre une avancée majeure en conception moléculaire d’adsorbants polymériques : la combinaison d’une structure supramoléculaire sélective et de fonctions ioniques actives permet d’obtenir une capture rapide, robuste et sélective des PFAS dans des conditions environnementales réalistes. Au-delà de son efficacité pratique, cette approche démontre le potentiel des réseaux polymériques à base de cyclodextrine comme solution industrielle et durable pour la dépollution des eaux contaminées par les composés fluorés persistants.
Nature Hydrogel luminescent auto-cicatrisant pour la détection ultra-sensible du formaldéhyde
Des chercheurs de l’Université Nationale de Taïwan ont conçu un hydrogel luminescent injectable et auto-réparable capable de détecter le formaldéhyde à des concentrations extrêmement faibles, ouvrant une nouvelle voie pour la surveillance environnementale en temps réel. Ce matériau innovant repose sur un réseau polymérique combinant une gélatine modifiée et un composé sucre–polydextran (PG/PDA), renforcé par des nanoparticules de laponite contenant des ions europium. Ces particules, Eu³⁺(TTA)@Lap, confèrent au gel ses propriétés optiques grâce à un « effet antenne » où les ligands organiques amplifient l’émission lumineuse du métal. Lors d’une exposition à des composés organiques volatils, la luminescence du gel varie de manière spécifique, permettant d’identifier les substances présentes. Le système se distingue par une sensibilité remarquable, détectant le formaldéhyde à partir de 39 parties par milliard, soit bien en dessous des seuils de sécurité fixés par l’OMS. Outre ses performances analytiques, l’hydrogel peut se régénérer après dommage et être injecté sous différentes formes, ce qui facilite son intégration dans des environnements complexes ou des dispositifs portables. Cette combinaison de luminescence, de flexibilité mécanique et de réversibilité chimique illustre le potentiel des nanocomposites polymériques intelligents pour la détection sélective de polluants gazeux. Elle ouvre la voie à des capteurs biocompatibles et autonomes dédiés à la prévention des risques sanitaires liés aux composés volatils dans l’air intérieur et industriel.
https://phys.org/news/2025-10-healable-hydrogel-ultra-sensitive-formaldehyde.html
Valorisation du PET en composants de supercondensateurs : une voie circulaire pour le stockage d’énergie
Des chercheurs ont mis au point une méthode thermique innovante permettant de transformer le poly(éthylène téréphtalate) issu de bouteilles à usage unique en électrodes et films séparateurs pour supercondensateurs tout-plastique. Ce procédé, présenté dans ACS Energy & Fuels, repose sur la conversion du PET en carbone conducteur par chauffage sous vide en présence d’hydroxyde de calcium, générant une poudre poreuse utilisée pour former des électrodes minces et performantes. En parallèle, de petits fragments de PET aplatis et microperforés par chauffage servent de films séparateurs, optimisant la conduction ionique dans l’électrolyte. Le dispositif obtenu, basé sur le principe des condensateurs à double couche électrique, affiche des performances équivalentes à celles de systèmes conventionnels à séparateur en fibre de verre, tout en étant plus économique et entièrement recyclable. Cette approche illustre une synergie entre valorisation des déchets plastiques et technologies de stockage d’énergie, ouvrant la voie à des supercondensateurs issus de matériaux circulaires. Selon les auteurs, cette stratégie pourrait être industrialisée à moyen terme, contribuant à réduire l’empreinte environnementale des dispositifs électrochimiques et à renforcer la durabilité des systèmes énergétiques utilisés dans la mobilité, l’électronique et les applications industrielles.
Vers des alternatives au PEG : de nouveaux polymères zwitterioniques pour la vectorisation lipidique
Cette étude met en lumière une innovation stratégique dans le domaine des nanoparticules lipidiques en proposant le remplacement des lipides PEGylés traditionnels par des polymères-lipides zwitterioniques et des polymères en brosse. Ces nouvelles architectures polymériques visent à surmonter les limites du polyéthylène glycol, notamment sa reconnaissance immunitaire croissante et la diminution d’efficacité lors d’administrations répétées. En combinant une neutralité de charge intrinsèque à une conformation dense et hydratée, les polymères zwitterioniques réduisent significativement l’adsorption de protéines plasmatiques et prolongent la stabilité colloïdale des particules, tout en favorisant une internalisation cellulaire plus efficace. Les polymères en brosse, grâce à leur organisation tridimensionnelle, améliorent la protection de la surface lipidique et optimisent la libération intracellulaire des charges thérapeutiques. Cette approche représente une évolution majeure vers des nanovecteurs plus biocompatibles et moins immunogènes, capables d’assurer une délivrance répétée sans perte d’efficacité. Sur le plan industriel, ces substituts du PEG ouvrent la voie à une nouvelle génération de formulations pour l’administration de vaccins, d’ARN messagers et de principes actifs biologiques, en répondant aux exigences croissantes de sécurité et de performance dans les biotechnologies pharmaceutiques.
Nature Lorem ipsum dolor sit amet, consectetur adipiscing elit. Sed posuere tincidunt quam sit amet viverra. Nam in consequat nulla. Nunc rhoncus orci vitae arcu sagittis, in auctor nibh posuere. Donec ut nulla id enim tempor feugiat.
Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
Lorem ipsum dolor sit amet, consectetur adipiscing elit. Etiam feugiat quis risus quis tempus. Morbi pharetra volutpat ligula ut placerat. Morbi sagittis ornare tellus, at molestie urna suscipit id. Praesent non est quis ante pretium ullamcorper. Lorem ipsum dolor sit amet, consectetur adipiscing elit. Vestibulum ante ipsum primis in faucibus orci luctus et ultrices posuere cubilia Curae; Integer sodales nisi justo, a varius nisi viverra accumsan. Quisque eleifend velit sed suscipit convallis. Donec ac facilisis massa. Donec euismod erat molestie nisi condimentum mattis. Nunc eu eros lacinia, vestibulum nibh vitae, varius magna. Aliquam erat volutpat. Suspendisse potenti.
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