Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Fusion hétérogène contrôlée cinétiquement entre nanoparticules polymères : vers un assemblage systémique non-équilibre
Des chercheurs ont récemment démontré que des populations distinctes de nanoparticules polymères, sans modification chimique de surface, peuvent fusionner entre elles selon un contrôle purement cinétique, ouvrant une nouvelle voie pour la manipulation nano-structurale des polymères. L’étude montre que la longueur des chaînes polymères — modulable par le procédé de synthèse — suffit à réguler l’étendue de la fusion entre nanoparticules issues de populations différentes, sans besoin d’unités de reconnaissance anisotropes ni de forces thermodynamiques spécifiques. Grâce à un marquage élémentaire et à l’utilisation de techniques d’imagerie cryogéniques combinées à la spectroscopie électronique, les auteurs ont mis en évidence que ce comportement de « communication » entre particules constitue un phénomène collectif — à l’échelle du système — comparable à des interactions biologiques de type fusion membranaire. Cette approche illustre comment des mécanismes purement physiques (mobilité des chaînes, entropie, dynamique de surface) peuvent suffire à orchestrer des architectures nanométriques complexes, sans recourir à une chimie sophistiquée de surface. La portée technologique de ces résultats est surtout conceptuelle : ils ouvrent la possibilité de concevoir des systèmes polymères auto-organisés, adaptables et potentiellement réactifs, basés sur la fusion contrôlée de nanoparticules — une stratégie prometteuse pour des applications en nanomatériaux, en délivrance ciblée, en assemblages hiérarchiques ou en matériaux à fonctionnalités dynamiques.
Memorandum Jean-Marie Catala
Jean-Marie Catala est arrivé au Centre de Recherches sur les Macromolécules (CRM) en 1972, pour y suivre l’enseignement de troisième cycle sur les polymères de l’Université Louis Pasteur de Strasbourg. Il a été accueilli dans l’équipe Synthèse Organique Macromoléculaire du Professeur Jean Brossas. Il y a préparé une thèse de troisième cycle, sur la synthèse de polymères téléchéliques à extrémités hydroperoxyde (soutenue en 1975), puis une thèse d’état, sur l’action de l’oxygène sur des oligomères et des polymères mono- et multi-carbanioniques (soutenue en 1980). Lors de ces premières études, il n’a pas réalisé que les synthèses des polymères ; il a aussi étudié les mécanismes réactionnels pour maîtriser chacune des étapes de la fonctionnalisation par des études cinétiques, bénéficiant particulièrement de discussions avec Gilbert Clouet. À une époque où cela n’était pas encore répandu, il utilisait déjà couramment plusieurs techniques de caractérisation telles que RMN, IR et CES. Cette attitude de chimiste consciencieux, il l’a conservée tout au long de sa carrière, c’est-à-dire jusqu’à son départ à la retraite, en 2012. lire plus…
Les Webinaires Matériaux : En préparation du congrès « Matériaux 2026 »
Aurélie CAYLA (ENSAIT, GEMTEX)
Professeure en chimie des matériaux depuis 2020, sa carrière est consacrée à l’élaboration, à la formulation et à la compréhension de la mise en forme des polymères sous forme filamentaire, ainsi qu’à leurs caractérisations associées.
Ses recherches récentes portent sur l’élaboration de filaments à partir de ressources biosourcés et/ou biodégradables dans des procédés de plasturgie des thermoplastiques (extrusion/filage), mais également des procédés en voie solvant de polymères naturels (voie humide). Ses activités s’intègrent dans divers domaines d’applications qui entrainent une variabilité de propriétés à développer à l’échelle du filament (antibactérien, ignifuge, conducteur d’électricité…). lire plus…
Polymères PEG imprimables en 3D : une nouvelle architecture bottlebrush pour hydrogels et élastomères hautement extensibles
Des chercheurs ont développé une nouvelle génération de matériaux polymères imprimables en 3D à partir de réseaux de polyéthylène glycol dont l’architecture moléculaire a été entièrement repensée pour surmonter la rigidité intrinsèque des PEG réticulés de manière classique. Leur approche s’appuie sur la conception dite bottlebrush pliable, dans laquelle un squelette polymère central porte de nombreuses chaînes latérales flexibles capables de se replier et de se déployer, stockant ainsi une réserve de longueur interne qui confère au réseau une extensibilité exceptionnelle sans rupture de cohésion. En initiant la polymérisation par exposition brève aux UV, l’équipe obtient des hydrogels et élastomères sans solvant dont la micro-organisation reste contrôlable via la géométrie du champ lumineux, permettant de fabriquer des architectures complexes, souples ou rigides, tout en préservant une grande déformabilité. Cette stratégie permet au PEG, déjà largement utilisé en biomédecine, d’adopter des propriétés mécaniques compatibles avec des structures plus volumineuses ou fonctionnelles, notamment des échafaudages dynamiques pour organes artificiels ou des matrices de délivrance thérapeutique. De plus, la biocompatibilité constatée ouvre la voie à des interfaces intracorporelles stables, tandis que la combinaison possible du PEG avec d’autres motifs chimiques laisse entrevoir une large palette de formulations. L’étude met également en avant le potentiel de ces réseaux pour les électrolytes polymères solides, où la synergie entre conductivité et grande extensibilité représente un atout pour les dispositifs de stockage d’énergie de nouvelle génération.
https://www.eurekalert.org/news-releases/1106291
Polymère pour une administration sans aiguille de l’insuline
Une équipe de chercheurs de Zhejiang University a mis au point une nouvelle architecture polymère capable de franchir la barrière cutanée intacte et de transporter l’insuline dans la circulation systémique, ouvrant une voie inédite vers l’administration sans aiguille. Le polymère, désigné poly[2-(N‑oxide‑N,N‑dimethylamino)ethyl methacrylate] (OP), exploite une bascule de charge : à la surface de la peau, où le pH est légèrement acide, il se charge positivement et interagit électrostatiquement avec les lipides négativement chargés de la couche cornée, ce qui lui permet de s’insérer entre les lipides et d’amorcer sa traversée de la peau. En pénétrant plus profondément vers un environnement neutre, OP passe en état zwitterionique neutre global, réduisant ses interactions avec les matrices lipidiques et facilitant ainsi sa diffusion vers les couches sous-cutanées et la circulation sanguine. Lorsqu’il est lié à l’insuline, ce système a permis chez des animaux diabétiques un abaissement de la glycémie comparable à une injection tout en ne provoquant pas d’irritation cutanée ni de dommages structuraux après des applications répétées. Cette avancée promet non seulement d’améliorer la qualité de vie des patients en réduisant la dépendance aux injections, mais elle ouvre également la voie à l’administration transdermique d’autres biomolécules de poids moléculaire élevé — peptides, protéines thérapeutiques — tout en incitant à repenser les architectures polymères et les interfaces biomédicales pour l’intérieur du corps.
IA et surfaces de membranes poreuses pour une filtration par affinité chimique
Une équipe a développé un matériau de membrane ultrafiltrante novateur capable de trier des molécules de taille identique mais de nature chimique différente grâce à une architecture de pores fonctionnalisés. Le procédé repose sur l’auto-assemblage de micelles de copolymères à blocs chimiquement distincts, mélangés puis transformés en films poreux dont la surface interne présente des motifs chimiques variés selon les micelles utilisées. L’identification et l’optimisation de cette organisation complexe ont été rendues possibles par l’usage de techniques d’imagerie par microscopie électronique couplées à un algorithme d’apprentissage automatique, tandis que des simulations moléculaires ont permis d’éclairer les règles gouvernant l’auto-assemblage ; cette approche révèle comment la chimie des pores — et non seulement leur taille — peut être programmée. Du point de vue moléculaire, l’architecture repose sur la juxtaposition sélective de domaines fonctionnels dans les parois de pores, ce qui modifie l’affinité des molécules entrantes et permet de discriminer celles qui présentent des groupements de surface différents. Cette avancée ouvre des perspectives technologiques importantes : produire par des procédés industriels existants des membranes ultrafiltrantes capables de séparer selon l’affinité chimique, ce qui pourrait révolutionner des secteurs tels que la bio-pharmacie, le traitement de l’eau, voire les capteurs et revêtements intelligents.
https://phys.org/news/2025-11-machine-membranes-chemical-affinity.html
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Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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Les partenaires
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Waters_logo_stacked_K_web-NEW
http://www.waters.com
arkema
http://www.coatex.com
LPMC
http://www.ispa.asso.fr
logo-ispa_coul_fond-fonce
http://www.ispa.asso.fr
ICS
https://www-ics.u-strasbg.fr/
Logo-ChemSuD
http://www.ispa.asso.fr
lrccp
http://www.ispa.asso.fr
hutchinson
http://www.hutchinson.com/fr
cnrs
http://www.ispa.asso.fr
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