Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Durabilité chimique des composites bio-polyamide renforcés en fibres de cellulose régénérée face aux milieux acides et basiques
Cette étude analyse la stabilité chimique du polyamide biosourcé PA5.10 et de ses composites renforcés par des fibres de cellulose régénérée (RCF), dans le but d’évaluer leur aptitude à remplacer les polyamides pétrosourcés dans des applications techniques exigeantes. Les échantillons, élaborés par extrusion bi-vis et moulage par injection, ont été exposés à divers environnements aqueux, acides, alcalins et organiques afin d’identifier les mécanismes de dégradation et les effets sur les propriétés mécaniques et structurales. Les résultats montrent que la dégradation hydrolytique constitue le principal facteur d’altération du polymère, se traduisant par des phénomènes de coupure de chaînes, de gonflement des fibres et de désadhésion à l’interface matrice-fibre. Les milieux acides et basiques accélèrent la scission des liaisons amide dans la matrice et la rupture des liaisons glycosidiques de la cellulose, provoquant un affaiblissement progressif du renfort et une perte de cohésion du composite. Les analyses FTIR et microscopiques confirment ces processus, tandis que les essais mécaniques mettent en évidence une baisse de résistance en traction corrélée à l’absorption d’humidité et à la dégradation chimique. Malgré cette sensibilité, les composites PA5.10/RCF présentent un comportement ductile et une densité réduite, constituant une alternative plus légère et à plus faible empreinte carbone que les composites à fibres de verre. Les auteurs soulignent toutefois la nécessité d’optimiser la formulation par l’ajout de stabilisants hydrolytiques ou de traitements de surface des fibres afin d’améliorer la durabilité de ces matériaux biosourcés dans des environnements chimiques sévères.
Nature Réseau PVA–SPPESK à volume libre optimisé et photothermie sélective pour des revêtements anti-buée durables et transparents
Les auteurs proposent une architecture polymère qui combine une matrice hydrophile à liaisons hydrogène (polyvinylalcool) et des segments sulfonés à géométrie torsadée non coplanaire (SPPESK) afin d’augmenter le volume libre interne sans épaissir le film, stabiliser l’adhésion interfaciale et maintenir la transparence; cette conformation favorise un maillage dense de liaisons H et engendre une distribution bimodale de cavités, couplant des pores « piégeurs » nanométriques (rétention d’eau non givrante) et des canaux de diffusion (apport rapide), ce qui supprime la nucléation de microgouttes au profit d’un film continu même sous cycles humidité/séchage; l’intégration de nanocristaux de bronze tungstate césium (CTB) ajoute une photothermie sélective UV/NIR tout en préservant la transmission visible, convertissant une part significative du spectre solaire en élévation locale de température pour prévenir ou résorber la buée sans alimentation électrique; la formulation, mise en œuvre par trempage, essorage ou racle, montre une forte robustesse mécanique (adhésion, anti-abrasion, anti-encrassement) et une compatibilité substrats rigides/flexibles, avec des essais en conditions réelles (verres correcteurs, pare-brise, serres) confirmant la constance d’optique et l’anti-buée prolongée; en reliant conception moléculaire (torsion, sulfonation) et ingénierie d’interface (brosses H, volume libre hiérarchisé, photothermie transparente), cette stratégie dépasse les limites des hydrophiles gonflants et des hydrophobes cassie-baxteriens, ouvrant la voie à des revêtements anti-buée pérennes, recyclables en service par la lumière ambiante et industrialisables à grande échelle.
Nature Syensqo met au point une technologie de recyclage chimique pour des polymères sulfonés circulaires
Le groupe Syensqo annonce une avancée majeure dans le domaine des polymères techniques avec le développement d’une technologie exclusive de recyclage chimique capable de dépolymériser efficacement les polymères sulfonés (PAES) afin d’en extraire des monomères purifiés réutilisables à l’infini. Cette innovation, issue de la gamme durable ECHO™, permet de transformer aussi bien les rebuts de production que les produits en fin de vie en matières premières de haute pureté, sans dégradation des performances. Les monomères régénérés peuvent être réincorporés dans les grades emblématiques de Syensqo — Udel® PSU, Radel® PPSU et Veradel® PESU — ou dans d’autres polymères thermoplastiques et formulations d’époxy, garantissant une véritable circularité moléculaire. En ciblant les marchés exigeants tels que la filtration, la santé ou l’aéronautique, l’entreprise renforce son leadership en matière de polymères durables à haute performance. Selon Floryan De Campo, vice-président Life Solutions, cette technologie marque une étape décisive vers la décarbonation et l’intégration accrue de matières recyclées dans les chaînes de valeur. En s’appuyant sur la coopération entre acteurs du tri, de la collecte et de la transformation, Syensqo trace la voie d’un modèle circulaire pour les polymères sulfonés, conciliant innovation industrielle et responsabilité environnementale.
Quand les polymères fondus racontent le cosmos
Le chercheur John Spevacek établit un parallèle fascinant entre la physique des polymères fondus et celle de l’univers, où la matière plastique devient une métaphore de l’espace-temps. Comme un polymère viscoélastique capable à la fois de couler et de stocker de l’énergie, l’espace-temps se révèle lui aussi fluide et élastique : sa viscosité se manifeste dans l’expansion issue du Big Bang, tandis que son élasticité se dévoile à travers les ondes gravitationnelles nées des collisions de trous noirs. Ces infimes vibrations traduisent la capacité du cosmos à se déformer puis se détendre, à la manière d’un plastique chauffé. Spevacek souligne ainsi que les mêmes outils mathématiques — tenseurs, équations de déformation, élasticité — servent autant à décrire un polymère en fusion qu’à comprendre la relativité d’Einstein, reliant de façon poétique la matière fondue aux profondeurs du temps et de l’espace.
Membranes sPEEK dopées aux liquides ioniques prototropes ouvrant la voie à des électrolytes polymères hautement conducteurs
Cette recherche explore une approche innovante pour concevoir des membranes électrolytes polymères capables de fonctionner au-delà de 100 °C dans les piles à combustible. En incorporant des liquides ioniques prototropes de différentes acidités dans une matrice de poly(éther-éther-cétone) sulfoné (sPEEK) réticulée, les chercheurs obtiennent des matériaux conjuguant stabilité thermique, conductivité protonique élevée et structure mécanique robuste. Le sPEEK, polymère fluorine-free à forte affinité hydrophile, assure une ancrage efficace des liquides ioniques tout en apportant ses propres sites donneurs de protons. Selon l’acidité du liquide ionique utilisé, le transport des protons s’opère par des mécanismes coopératifs impliquant H₃O⁺, améliorant la conduction même en conditions de faible humidité. Les observations morphologiques révèlent toutefois une microstructure hétérogène suggérant des pertes partielles d’électrolyte, un point clé à optimiser pour une meilleure durabilité. En combinant chimie des polymères et électrochimie des liquides ioniques, cette approche ouvre la voie à des électrolytes hybrides stables, efficaces et respectueux de l’environnement pour les PEMFC de nouvelle génération.
Nature Membrane réticulée à motifs 12-couronne-4 pour une capture sélective et régénérable du lithium en milieu aqueux
Un monomère diallylammonium portant un motif 12-couronne-4 a été synthétisé puis polymérisé par cyclopolymérisation radicalaire et réticulé, avec insertion contrôlée de SO₂, afin d’obtenir des résines insolubles dotées de cavités chélatantes accordées au Li⁺. Cette architecture conjugue reconnaissance hôte–invité des éthers couronne, sites ammonium répartis dans le réseau et segments sulfone qui rigidifient et polarisent la matrice, générant une texture mésoporeuse à grande surface favorable aux transferts. Les tests en solutions binaires confirment une forte sélectivité vis-à-vis de Na⁺ et K⁺ et un avantage sur Mg²⁺ à concentrations équivalentes, tandis que FTIR et XPS indiquent l’implication des liaisons éther dans la complexation. Régénérable par désorption acide, cette plateforme polymère offre une voie crédible pour la récupération durable du lithium et l’épuration d’effluents.
Nature Lorem ipsum dolor sit amet, consectetur adipiscing elit. Sed posuere tincidunt quam sit amet viverra. Nam in consequat nulla. Nunc rhoncus orci vitae arcu sagittis, in auctor nibh posuere. Donec ut nulla id enim tempor feugiat.
Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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Les partenaires
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hutchinson
http://www.hutchinson.com/fr
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http://www.waters.com
lrccp
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arkema
http://www.coatex.com
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LPMC
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ICS
https://www-ics.u-strasbg.fr/
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cnrs
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