Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Effervescence réglementaire et bascule circulaire des polymères entre emballage, BTP et pneumatiques
Une étude récente met en lumière l’accélération simultanée des contraintes normatives et des réponses technologiques dans les filières des polymères et des élastomères, où compétitivité et décarbonation s’imbriquent plutôt qu’elles ne s’opposent. Dans l’emballage, le débat se cristallise autour de l’adaptation du cadre national au règlement européen relatif aux emballages et aux déchets d’emballages (PPWR), avec, en toile de fond, un resserrement progressif des conditions de mise sur le marché des plastiques à usage unique. Parallèlement, dans les travaux publics, l’innovation produit s’incarne dans une conduite d’eau potable revendiquée comme fortement décarbonée, fondée sur une matrice polymère biosourcée et sécurisée par une certification de traçabilité (ISCC+), illustrant la montée en puissance de matières premières renouvelables compatibles avec les exigences d’infrastructures. Côté caoutchoucs et pneumatiques, la dynamique passe autant par l’expansion internationale que par l’intégration de savoir-faire : partenariats et acquisitions visent des formulations de haute performance pour joints et applications fonctionnalisées, tandis que le recyclage chimique par pyrolyse progresse vers des capacités industrielles, en convertissant des élastomères réticulés en fractions valorisables comme ressources de circularité.
L’Usine Nouvelle Sonifier la solvatation pour décoder l’effondrement conformationnel du poly(N-isopropylacrylamide)
Des chercheurs ont déchiffré, à partir de simulations moléculaires longues et d’une analyse par sonification, la manière dont l’eau gouverne l’effondrement conformationnel de poly(N-isopropylacrylamide) en solution aqueuse. Ce polymère thermoréactif, soluble à basse température puis précipitant lorsqu’il devient plus hydrophobe à température plus élevée, sert de plateforme à des matériaux « intelligents », mais la contribution exacte du solvant restait difficile à isoler tant le réseau de liaisons hydrogène se reconfigure sans cesse. En attribuant des signatures sonores distinctes aux différents motifs de liaison, l’équipe montre que la contraction ne s’organise pas principalement par contacts directs entre segments de chaîne : elle est au contraire orchestrée par des « ponts d’eau », où une molécule d’eau relie deux régions de PNIPAM par liaisons hydrogène et impose une topologie transitoire, corrélée et collective. Parallèlement, une interaction locale atypique, impliquant l’alignement de liaisons N–H, accompagne la structuration des segments latéraux. Cette lecture, qui replace le solvant au cœur de l’architecture dynamique du polymère, fournit des règles de conception plus fines pour ajuster réversibilité, cinétique et sélectivité de réponse dans des hydrogels, capteurs et dispositifs biomédicaux fondés sur des transitions coil-globule pilotées par la solvatation.
https://phys.org/news/2026-02-polymers-collapse-bridges.html
Isocyanates biosourcés : le PDI comme levier de réticulation pour des revêtements polyuréthane plus durables
Une étude récente met en lumière la faisabilité d’une substitution partielle des isocyanates d’origine fossile dans les revêtements polyuréthane, longtemps dominés par le diisocyanate d’hexaméthylène, en s’appuyant sur un diisocyanate biosourcé de pentaméthylène fourni sous forme de trimères intégrables dans des formulations existantes. La filière amont repose sur des matières premières renouvelables transformées en pentaméthylènediamine, puis en motifs isocyanates susceptibles d’augmenter la densité de réticulation lors de la réaction avec des polyols, qu’il s’agisse de résines polyuréthane à base de polyester polyol ou de dispersions polyuréthane associées à un polyacrylate polyol. Les performances de surface s’en trouvent modifiées de manière cohérente : une cinétique de durcissement plus réactive favorise une rigidification du réseau, ce qui se traduit par une résistance accrue aux rayures et à l’abrasion, ainsi que par une formation de film plus uniforme, donnant des surfaces plus lisses et plus brillantes, avec une hydrophobicité légèrement renforcée. En contrepartie, la stabilité thermique apparaît un peu moins favorable, et les mécanismes de vieillissement divergent, le PDI montrant plutôt des signatures d’oxydation et de réarrangement superficiel après usure, là où le système fossile manifeste davantage de scissions de chaîne. Ces résultats dessinent une voie de transfert industriel pragmatique, moyennant des ajustements de formulation et de conditions de cure, pour proposer des finitions à forte valeur d’usage tout en réduisant la dépendance au carbone fossile.
Du caoutchouc en fin de vie à la ressource : fonctionnalisation du polybutadiène pour une circularité crédible
Une étude récente met en lumière la difficulté intrinsèque de valoriser les déchets de caoutchouc synthétique, dont la vulcanisation transforme des chaînes de poly(diène) en réseaux tridimensionnels densément réticulés par des ponts soufrés, souvent noyés dans des composites chargés qui entravent diffusion, sélectivité et contrôle de l’architecture macromoléculaire. L’analyse propose un panorama critique des stratégies de modification post-polymérisation, conçues non pas pour dépouiller le matériau par dépolymérisation, mais pour exploiter l’insaturation du squelette afin d’introduire des fonctions d’interface, des motifs ioniques, des sites dynamiques ou des points d’ancrage réticulables. Les voies catalytiques (hydro-fonctionnalisation, métathèse, hydrogénation, hydrosilylation) sont discutées au prisme de leur robustesse en présence d’impuretés, tandis que des alternatives sans métal ou sans catalyse (réactions « click », oxydations sélectives, greffages électrophiles, approches en phase solide) illustrent l’arbitrage permanent entre efficacité, innocuité et simplicité de procédé. Pour les réseaux vulcanisés, des exemples de désassemblage chimiosélectif ou de conversion en matériaux fonctionnels soulignent l’intérêt d’une ingénierie guidée par des métriques, intégrant mécanochemie, apprentissage automatique et analyse de cycle de vie. L’ensemble dessine une feuille de route vers des technologies industrialisables capables de requalifier les élastomères usagés en intermédiaires à forte valeur pour adhésifs, résines et formulations circulaires.
Alcènes hyperpyramidalisés dans des cages moléculaires : vers des briques 3D au-delà des règles classiques
Une étude récente met en lumière la possibilité de forcer une double liaison carbone–carbone à adopter une géométrie franchement tridimensionnelle, à rebours de la planarité qui gouverne habituellement les alcènes, en générant des motifs de type cubène et quadricyclène au sein de cages fortement contraintes. La stratégie de synthèse repose sur la préparation de précurseurs stables portant des substituants silylés et des groupes partants judicieusement positionnés ; l’activation par des sels de fluorure déclenche alors, in situ, la formation fugace de l’alcène « tordu », dont la réactivité élevée impose une interception immédiate par des partenaires piégeurs pour aboutir à des produits élaborés autrement difficiles d’accès. Sur le plan mécanistique, la distorsion se traduit par une pyramidation extrême des carbones vinyliques, affaiblissant le recouvrement π et conduisant à un ordre de liaison fractionnaire, intermédiaire entre simple et double, ce que confortent des analyses computationnelles et des indices expérimentaux indirects malgré l’impossibilité d’isoler l’intermédiaire. En élargissant le répertoire des architectures rigides et compactes disponibles, cette chimie fournit des « blocs de construction » 3D prometteurs pour l’assemblage de squelettes moléculaires inédits, directement transposables aux besoins de la découverte de médicaments et, plus largement, de la synthèse fine à forte valeur ajoutée.
https://scitechdaily.com/ucla-chemists-have-created-impossible-3d-bonds-that-shouldnt-exist/
Film microperforé en copolyester élastomère pour prolonger la fraîcheur des produits végétaux
Une étude récente met en lumière une technologie de film d’emballage destinée aux fruits, légumes et fleurs qui vise à remplacer l’atmosphère modifiée « injectée » par une atmosphère auto-régulée, générée in situ par l’équilibre entre respiration du végétal et transferts gazeux à travers la paroi polymère. Le matériau s’appuie sur un copolyester thermoplastique à comportement élastomère, formulé pour conjuguer perméation sélective et ténacité, puis mis en forme en film et doté d’une microperforation laser d’une précision élevée ; l’ajustement fin de la densité et de la géométrie des perforations module simultanément la diffusion de l’oxygène et du dioxyde de carbone, de façon à instaurer un milieu appauvri en oxygène qui ralentit les processus métaboliques, limite les phénomènes oxydatifs et freine la croissance de microorganismes aérobies. Parallèlement, une perméabilité élevée à la vapeur d’eau, combinée à une barrière suffisante pour retenir l’humidité utile, évite à la fois la condensation propice aux moisissures et le dessèchement responsable des pertes de qualité. L’absence de réticulation chimique préserve la recyclabilité du film, tandis que la résistance à la perforation autorise son emploi en doublures de bacs et en housses logistiques, ouvrant une voie industrialisable pour réduire le gaspillage alimentaire et verdir le transport longue distance.
https://www.plasticstoday.com/packaging/packaging-film-extends-fresh-produce-shelf-life
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Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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Les partenaires
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Logo-ChemSuD
http://www.ispa.asso.fr
LPMC
http://www.ispa.asso.fr
Waters_logo_stacked_K_web-NEW
http://www.waters.com
cnrs
http://www.ispa.asso.fr
logo-ispa_coul_fond-fonce
http://www.ispa.asso.fr
lrccp
http://www.ispa.asso.fr
hutchinson
http://www.hutchinson.com/fr
ICS
https://www-ics.u-strasbg.fr/
arkema
http://www.coatex.com
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