Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Tétrafonctions cyclobutanes pour moduler la ténacité des réseaux polymères
Des chercheurs ont démontré qu’en intégrant dans un réseau polymère simple des jonctions méchanoréactives à base de cyclobutanes tétrafonctionnels (TCB), il devient possible de réguler la ténacité sans changer la composition chimique ou la topologie du réseau. Ces mécanophores TCB sont activables uniquement sous contrainte multidirectionnelle et modifient localement la continuité des chaînes dans le réseau, permettant d’augmenter ou de réduire la tenue mécanique d’un gel end-linké. Le concept de « continuité de brin réseau » émerge ainsi comme un descripteur topologique pour interpréter comment la réactivité couplée à la contrainte se traduit en propriété macroscopique. Cette avancée offre un cadre nouveau pour designer des réseaux polymères simples mais adaptables, ouvrant des perspectives pour des gels hautement performants en rupture contrôlée, fatigue ou contraintes dynamiques.
Nature Contrôle réversible de la séparation liquide-liquide par moteurs moléculaires rotatifs dans des assemblages supramoléculaires
Des chercheurs ont démontré qu’un monomère moléculaire intégrant un moteur rotatif gouverné par la lumière peut piloter la phase séparée liquide-liquide (LLPS) de ses assemblages supramoléculaires, en passant par plusieurs états non-à-l’équilibre. La rotation unidirectionnelle induite par irradiation et inversion thermique modifie successivement le moment dipolaire et la capacité de liaison hydrogène du moteur, ce qui fait varier la température critique de séparation et entraîne la formation ou la dissolution de gouttelettes aux interfaces internes. Cette stratégie permet une modulation orthogonale — par la température et la lumière — de la morphologie et de la dynamique des phases, ouvrant ainsi une voie nouvelle à la conception de matériaux mous adaptatifs, capables de capturer puis relâcher des composants selon stimuli externes.
Nature Ateliers Prospective 2026 : Réservez la date !
Polymères pour batteries Metal ion
Date : 4 Février 2026
La filière européenne des batteries vit une phase stratégique, produire des batteries metal ion hautes performances, compétitives, durables et souveraines.
Les polymères y jouent un rôle déterminant, les binders d’électrodes jusqu’aux séparateurs et électrolytes solides.
Ils conditionnent, en partie, la productivité des lignes, la sécurité, la durabilité des cellules metal-ion. lire plus…
L’intelligence artificielle améliore la détection des microplastiques par spectroscopie infrarouge
Des chercheurs des Instituts de physique de Hefei (Académie chinoise des sciences) ont développé une méthode d’apprentissage profond permettant de classer les microplastiques mixtes avec une précision de 98 %, une avancée majeure pour la surveillance environnementale. Publiée dans le Microchemical Journal, leur approche combine un réseau neuronal convolutionnel à double branche avec un mécanisme d’attention (CBAM), inspiré des systèmes cognitifs humains. Chaque branche du réseau traite différentes composantes spectrales issues de la spectroscopie infrarouge, tandis que le module CBAM identifie successivement les canaux et régions spatiales les plus pertinents avant de générer une carte d’attention pondérée, affinant ainsi les caractéristiques extraites. Cette architecture hybride permet de mieux distinguer les signatures complexes des mélanges de polymères, souvent altérées par les variations de composition. L’analyse visuelle via Grad-CAM met en évidence les zones spectrales clés exploitées par le modèle, apportant une interprétation physique des décisions de l’IA. Cette méthode surpasse largement les algorithmes classiques de classification spectrale, ouvrant la voie à des systèmes automatisés de tri et de suivi des microplastiques dans les milieux aquatiques ou atmosphériques. En intégrant la puissance de l’attention neuronale et de la vision spectrale, cette innovation rapproche l’analyse environnementale d’une surveillance en temps réel, fiable et reproductible des polluants plastiques à l’échelle microscopique.
https://phys.org/news/2025-11-ai-method-boosts-microplastic-classification.html
Transformation réversible CO₂-induite de polymères souples en plastiques rigides et fluorescents
Cette étude démontre la conception de polymères nanostructurés capables de changer d’état mécanique et optique sous l’action du dioxyde de carbone, ouvrant la voie à une valorisation fonctionnelle de ce gaz. Les chercheurs ont élaboré des élastomères constitués de polyéthylèneimine (PEI) vitrifiable par CO₂ et de polydiméthylsiloxane (PDMS) perméable au CO₂, formant une morphologie à séparation de phases nanométrique. L’exposition au CO₂ entraîne la formation de carbamates et d’acides carbamiques qui réticulent densément la phase PEI, transformant instantanément un matériau souple (module de l’ordre du MPa) en plastique rigide (de l’ordre du GPa). Cette vitrification réversible s’accompagne d’une augmentation marquée du module d’élasticité, d’une perte d’adhérence et d’une réduction du frottement de surface, tout en amplifiant fortement la fluorescence bleue du polymère. La combinaison de la diffusion rapide du CO₂ à travers le PDMS et de la réactivité du PEI assure un déclenchement homogène et cyclable du durcissement, stable à température ambiante mais annulé par chauffage. Le phénomène permet également de visualiser et d’enregistrer des motifs luminescents réversibles, suggérant des applications dans les dispositifs de détection, d’affichage et de stockage optique. Ces matériaux multifonctionnels exploitent simultanément la capture, la réactivité et la transduction du CO₂, établissant un concept inédit de polymères « CO₂-curables » capables de convertir une molécule environnementale en stimulus mécanique et optique pour les technologies intelligentes.
Nature Réseaux polymères multicomposants tissés par nœuds intriqués asymétriques de type chaîne-et-trame
Les auteurs introduisent une stratégie de « tissage moléculaire » pour intégrer à l’échelle macromoléculaire deux polymères a priori peu compatibles, un polyuréthane flexible (PU) et une résine époxy rigide (EP). Ils conçoivent d’abord une chaîne de PU portant des ligands tridentates, puis génèrent des nœuds intriqués asymétriques en coordonnant ces sites à des ligands monodentates via des centres palladium(II). Ces nœuds, analogues moléculaires de croisements chaîne–chaîne d’un textile, servent ensuite de points de croissance pour la polymérisation de l’époxy, construisant un réseau WPU-EP dans lequel segments souples et rigides sont entremêlés de façon contrôlée. Les entanglements dynamiques associés à ces nœuds coordonnés assurent à la fois dissipation d’énergie (rupture/réformation des liaisons de coordination, glissement des chaînes) et maintien d’un squelette topologique continu, ce qui se traduit par une combinaison inhabituelle de grande déformabilité, forte résistance mécanique et excellente résilience sous chargements cycliques. La comparaison avec des réseaux références purement covalents ou supramoléculaires montre que l’entrelacement topologique améliore à la fois la compatibilité PU/EP, la stabilité du réseau et l’adhésion structurale, jusqu’à des applications de type adhésifs de haute performance. En modulant la densité de nœuds et la fraction époxy, les propriétés mécaniques et l’amortissement peuvent être ajustés finement, illustrant le potentiel des architectures « tissées » inspirées du macroscopique pour l’ingénierie de réseaux polymères multicomposants à propriétés mécaniques et adhésives sur mesure.
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Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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