Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Ingénierie de nanovecteurs furtifs à l’architecture biomimétique pour l’immunothérapie ciblée
Une étude récente met en lumière une stratégie d’encapsulation avancée visant à surmonter les limitations pharmacocinétiques des immunomodulateurs systémiques grâce au développement de revêtements polymères de « super-furtivité ». Cette approche repose sur l’auto-assemblage de copolymères à blocs amphiphiles formant une architecture micellaire cœur-coquille, dont la couronne hydrophile est constituée d’une brosse polymère dense, potentiellement de nature zwitterionique ou pseudo-peptidique. Cette interface macromoléculaire, caractérisée par une hydratation de surface exceptionnelle et une entropie conformationnelle élevée, génère une barrière stérique robuste qui inhibe drastiquement l’adsorption non spécifique des protéines plasmatiques, phénomène connu sous le nom d’opsonisation. En prévenant ainsi la reconnaissance et la séquestration rapide par le système réticulo-endothélial, ces nanotransporteurs bénéficient d’un temps de circulation sanguine considérablement prolongé. Parallèlement à cette protection passive, la fonctionnalisation de surface permet un ciblage actif, favorisant une accumulation préférentielle au sein du microenvironnement tumoral via l’effet de perméabilité et de rétention (EPR). Cette technologie de camouflage moléculaire, en découplant la toxicité systémique de l’efficacité thérapeutique , offre une plateforme robuste pour la délivrance contrôlée d’agents biologiques fragiles, marquant une étape décisive vers des traitements oncologiques de précision à index thérapeutique optimisé.
https://phys.org/news/2026-02-exploring-immune-drugs-coated-stealth.html
Synthèse de polyuréthanes sans isocyanate par voie dicarbamate assistée au dioxyde de carbone
Des chercheurs ont franchi un jalon décisif dans la chimie des polymères durables en développant un procédé de synthèse permettant l’obtention de polyuréthanes (PU) de haute performance sans recourir aux isocyanates toxiques traditionnels. Cette approche novatrice repose sur l’emploi de dicarbamates comme intermédiaires réactionnels clés, synthétisés par la valorisation catalytique du dioxyde de carbone, substituant ainsi les précurseurs pétrochimiques dangereux habituels. Contrairement aux voies alternatives existantes, telles que l’aminolyse des cyclocarbonates qui génère des groupements hydroxyles pendants modifiant la structure, cette nouvelle méthode aboutit à une architecture macromoléculaire strictement identique à celle des polyuréthanes conventionnels. Le mécanisme de polymérisation, opérant par transuréthanisation contrôlée, permet de conserver intégralement les propriétés physico-chimiques d’origine, notamment la flexibilité, la résistance mécanique et la stabilité thermique. Cette homologie structurale assure une compatibilité directe avec les chaînes de valeur industrielles existantes, autorisant une substitution « drop-in » sans altération des performances applicatives. En éliminant les risques sanitaires liés à l’exposition aux isocyanates et en réduisant l’empreinte carbone globale via l’incorporation de gaz à effet de serre, cette technologie ouvre des perspectives immédiates pour la fabrication sécurisée de dispositifs médicaux critiques et d’adhésifs techniques, réconciliant ainsi exigence industrielle et innocuité environnementale.
https://www.specialchem.com/plastics/news/researchers-develop-isocyanate-free-polyurethane
Stratégie de nanostratification biodégradable pour l’ingénierie des films d’emballage barrières
Une nouvelle initiative technologique majeure vise à révolutionner le secteur du conditionnement alimentaire et médical par le déploiement de films polymères nanostructurés alliant haute performance barrière et biodégradabilité programmée. S’appuyant sur une technologie de coextrusion de pointe développée en collaboration académique, ce procédé permet l’assemblage précis d’une multitude de strates polymères à l’échelle nanométrique, générant ainsi des métamatériaux aux propriétés physico-chimiques modulables sans recourir aux mélanges fondus traditionnels souvent hétérogènes. Cette architecture lamellaire sophistiquée offre une maîtrise exceptionnelle de la perméabilité moléculaire, conférant au matériau une résistance supérieure à l’oxygène et à la vapeur d’eau tout en renforçant sa ténacité mécanique face aux contraintes de transformation industrielle. En substituant les emballages multicouches conventionnels, notoirement difficiles à recycler, par ces structures fonctionnelles capables de se dégrader intégralement en fin de vie sans générer de résidus microparticulaires persistants, cette approche constitue une avancée décisive vers une économie circulaire des plastiques souples, réconciliant impératifs de conservation longue durée et innocuité environnementale.
Valorisation de régénérés d’EPDM dévulcanisés dans les matrices élastomères : impact structural et résilience thermo-oxydante
Une investigation récente scrute les répercussions physico-chimiques de l’incorporation de caoutchouc éthylène-propylène-diène monomère (EPDM) dévulcanisé au sein de formulations élastomères vierges, dans une optique de circularité des matériaux techniques. L’étude démontre que l’introduction de ces charges régénérées, obtenues par la rupture sélective des ponts sulfures, altère significativement la cinétique de réticulation en catalysant le processus de durcissement, tout en induisant une hétérogénéité topologique au sein du réseau macromoléculaire tridimensionnel. Cette reconfiguration structurelle, exacerbée par la présence de soufre résiduel actif, se traduit macroscopiquement par une rigidité accrue au détriment des propriétés ultimes en traction, révélant une compétition entre la densité de réticulation et la mobilité segmentaire. Toutefois, les analyses de vieillissement accéléré mettent en exergue une stabilité thermo-oxydante remarquable des composites hybrides, dont la cinétique de dégradation ne présente aucune accélération délétère par rapport aux standards de référence, validant ainsi l’intégrité du squelette polymère recyclé. Par ailleurs, des ajustements formulationnels ciblés permettent de restaurer partiellement l’équilibre des propriétés mécaniques en optimisant la dispersion des phases et les interactions interfaciales. Ces résultats confirment le potentiel industriel de ces matériaux recyclés pour des applications durables, sous réserve d’une maîtrise rigoureuse de la stœchiométrie et de l’architecture du réseau.
https://www.nature.com/articles/s41598-026-36961-w
Nouvelle résine polyphénylène sulfure flexible et sans PFAS à haute performance ignifuge
Une avancée significative dans l’ingénierie des super-thermoplastiques a été réalisée par Toray Industries avec la mise au point d’une résine polyphénylène sulfure (PPS) inédite, capable de conjuguer flexibilité mécanique et ignifugation intrinsèque sans recourir aux substances per- et polyfluoroalkylées (PFAS). L’architecture du matériau repose sur une technologie de contrôle microstructurel propriétaire (« Nanoalloy »), permettant la dispersion nanométrique homogène d’un élastomère oléfinique au sein de la matrice polymère cristalline, surmontant ainsi le compromis historique qui liait l’ajout de souplesse à une dégradation de la tenue au feu. Cette morphologie de phase contrôlée confère au composite une résilience exceptionnelle aux contraintes thermiques et chimiques, tout en garantissant un niveau d’auto-extinction conforme aux standards de sécurité les plus sévères, surpassant les performances des grades flexibles conventionnels. En offrant une alternative allégée et économiquement compétitive aux fluoropolymères traditionnels, cette innovation cible stratégiquement les applications critiques de la mobilité électrique et de l’industrie des semi-conducteurs, telles que les tuyauteries de refroidissement et l’isolation de câblage, promettant une simplification des processus d’assemblage et une conformité anticipée aux futures régulations environnementales.
Catalyse orthogonale acide-base pour l’élaboration de polyesters aromatiques recyclables à haute masse molaire
Une nouvelle approche permet de surmonter les limitations synthétiques historiques associées à la copolymérisation par ouverture de cycle des époxydes acidosensibles, tels que l’oxyde de styrène, avec l’anhydride phtalique. En déployant un système catalytique couplant un acide de Lewis organoboré à une base phosphazène stériquement encombrée, cette stratégie inhibe efficacement le réarrangement de Meinwald, un processus d’isomérisation parasite auto-entretenu par les impuretés acides qui restreignait jusqu’alors la croissance des chaînes. Ce contrôle chimiosélectif rigoureux autorise l’obtention de polyesters aromatiques présentant des masses molaires exceptionnelles et une distribution étroite, traduisant une architecture macromoléculaire homogène. Les matériaux résultants manifestent des propriétés thermomécaniques de premier plan, notamment une rigidité élevée et une stabilité thermique comparable aux standards des résines polystyrène, tout en conservant une processabilité thermoplastique aisée. Parallèlement à ces attributs structuraux, l’étude démontre la circularité intégrale de ces polymères, qui peuvent subir une dépolymérisation chimique quasi-quantitative catalysée par des acides, régénérant ainsi les monomères constitutifs pour un nouveau cycle de vie. Cette innovation offre une alternative crédible et durable aux polyoléfines conventionnelles, réconciliant haute performance et recyclabilité chimique dans le domaine des plastiques de commodité.
https://www.nature.com/articles/s41467-026-69201-w
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Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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Les partenaires
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cnrs
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ICS
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Logo-ChemSuD
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lrccp
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arkema
http://www.coatex.com
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http://www.waters.com
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