Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Atomes isolés axialisés pour convertir des polluants chlorés en oligomères valorisables
Des chercheurs ont conçu un catalyseur à atomes isolés de fer, logé dans une matrice carbonitrure et doté d’une coordination axiale azotée, afin d’imposer une sélectivité réactionnelle rarement atteinte lors du traitement oxydant de micropolluants organochlorés. L’architecture de site actif, inspirée d’une poche de liaison enzymatique, pilote l’activation du peroxymonosulfate vers la formation d’un complexe de surface électrophile, qui opère par transfert d’électrons à courte portée plutôt que par chimie radicalaire diffuse. L’extraction électronique du 2,4,6-trichlorophénol génère des intermédiaires cationiques transitoires, puis des espèces hydroxylées hautement réactives ; celles-ci favorisent une substitution nucléophile des liaisons C–Cl, tout en multipliant les fonctions phénoliques disponibles pour la réticulation. La cascade intégrée déchloration–hydroxylation–polymérisation oriente alors la croissance vers des liaisons C–O, conduisant majoritairement à des poly(éthers phényléniques) réticulés qui s’accumulent sous forme solide, au lieu d’être minéralisés. Parallèlement, le microenvironnement hydrophobe/polaire limite l’empoisonnement du site par les produits, ce qui stabilise l’activité en fonctionnement continu. Cette chimie ouvre une voie technologique crédible d’« upcycling » : dépolluer des effluents tout en générant des précurseurs polymères transformables en plastiques utilisables à l’échelle industrielle.
Formation de film en photovoltaïque organique
Une étude récente met en lumière qu’une maîtrise conjointe de l’agrégation en solution et de la compatibilité donneur–accepteur constitue le levier déterminant pour hisser des polymères conjugués linéaires, pourtant peu complexes, vers des performances de premier plan en cellules solaires organiques. Des copolymères thiazolothiazole linéaires à chlorination graduée de la chaîne principale sont conçus afin de moduler finement les interactions interchaînes et l’énergie de surface, la chloration introduisant des contacts non covalents de type Cl···S et Cl···π qui stabilisent la planéité conformationnelle, renforcent la pré-agrégation et orientent la cristallisation. Cette ingénierie moléculaire ajuste en parallèle la cinétique de formation du film : une agrégation trop faible conduit à un mélange excessif, tandis qu’une agrégation trop marquée expulse l’accepteur lors du séchage et induit une séparation de phases grossière ; à l’inverse, une chlorination intermédiaire impose un régime cinétique où la solidification séquentielle des constituants construit un réseau bicontinu interpénétré, à domaines pertinents et forte pureté de phase. Il en résulte une dissociation excitonique rapide, des voies de transport de charges continues et une recombinaison atténuée, ouvrant une trajectoire crédible vers des modules à bas coût compatibles avec des procédés de dépôt en solution et des formulations plus durables.
Nanoparticules de lignine pour des papiers barrière recyclables capables de rivaliser avec les emballages plastiques
Une étude récente met en lumière une stratégie de revêtement destinée à lever le compromis classique entre performance barrière et fin de vie des papiers d’emballage. L’approche repose sur une émulsion de Pickering huile-dans-eau dont la stabilité est assurée par des nanoparticules de lignine amphiphiles, adsorbées de façon robuste à l’interface, évitant le recours à des tensioactifs de synthèse. La phase aqueuse contient un polymère filmogène hydrophile, le poly(alcool vinylique) (PVA), qui densifie la couche par un réseau de liaisons hydrogène et renforce simultanément la cohésion mécanique ainsi que la résistance aux corps gras, tandis qu’un acide gras biosourcé, l’acide stéarique, constitue la phase hydrophobe et confère une forte déperlance. Déposée sur le substrat cellulosique, l’émulsion colmate la porosité et forme un film continu, compact et synergique, améliorant nettement la tenue à l’eau, l’anti-graissage et la résistance en milieu humide. À l’inverse des papiers laminés, la couche reste compatible avec un recyclage par repulpage à l’eau chaude : le PVA se solubilise, l’acide gras se redisperse et les nanoparticules se libèrent, permettant une récupération propre des fibres. La biodégradation en sol est également rapportée comme effective sur une échelle de temps courte, avec un intérêt direct pour l’emballage alimentaire, où la maîtrise des transferts de vapeur d’eau contribue à préserver la fraîcheur, ouvrant la voie à des alternatives industrialisables aux enductions plastiques.
Comprendre la gélification des poloxamères près de la température physiologique
Une étude récente met en lumière les mécanismes par lesquels des solutions de poloxamères, excipients thermosensibles couramment mobilisés pour la gélification in situ, basculent d’un état fluide injectable vers un gel stable au contact du corps. En s’appuyant sur des mélanges de poloxamer 407 (P407) et de poloxamer 188 (P188), le travail relie explicitement l’auto-assemblage moléculaire à l’émergence de propriétés rhéologiques macroscopiques : l’évolution depuis des chaînes isolées vers des micelles, puis leur empilement en organisations ordonnées de type réseau micellaire densifié, est corrélée aux signatures calorimétriques et à la montée de rigidité associée à la transition sol–gel. Le rôle de P188 apparaît ambivalent et fortement dépendant de sa proportion : à faible teneur, il perturbe le compactage de P407, déplaçant la gélification vers des conditions plus exigeantes; à l’inverse, lorsqu’il devient prépondérant, il concurrence l’hydratation de P407, accélère sa déshydratation et favorise la nucléation de micelles fines, dont le sur-empilement induit une gélification plus facile. Cette compréhension mécanistique dépasse l’optimisation empirique des formulations et ouvre la voie à des gels à gélification prédictible pour des systèmes de libération prolongée en thérapeutiques localisées, avec des prolongements crédibles vers les cosmétiques, l’alimentaire et des matériaux fonctionnels sensibles à la température.
https://phys.org/news/2026-01-smart-polymer-solutions-transition-gels.html
Capteurs de gaz OFET biodégradables guidés par la séparation de phase P3HT/PBS
Une étude récente met en lumière une stratégie de films polymères mélangés pour des capteurs de gaz à transistors à effet de champ organiques (OFET) conciliant performance et fin de vie plus sobre. Le cœur du dispositif repose sur l’association d’un semi-conducteur π-conjugué largement employé, le poly(3-hexylthiophène) (P3HT), avec un polyester biodégradable, le poly(butylène succinate) (PBS), afin de conférer à la couche active une flexibilité accrue et une dégradabilité en milieu marin tout en maintenant une conduction exploitable. L’originalité tient à une ingénierie des solvants qui pilote la morphologie : selon le système solvant, la séparation de phase bascule d’un régime plutôt horizontal, générateur d’une topographie hétérogène, à une séparation de phase verticale qui homogénéise la surface et stabilise la réponse électrique même lorsque la fraction de PBS devient très majoritaire. Cette architecture hiérarchisée influe directement sur la transduction chimiorésistive : l’enrichissement en PBS renforce la sensibilité aux gaz oxydants ciblés, avec une sélectivité marquée envers le NO2 par rapport à d’autres analytes, tout en atténuant les dérives associées à l’humidité et à l’oxygène. En visant des procédés de dépôt compatibles avec des substrats courants et des usages jetables, cette approche esquisse une électronique de détection à grande échelle susceptible de réduire concrètement le flux de déchets électroniques.
https://phys.org/news/2026-01-biodegradable-polymers-eco-friendly-high.html
Recyclage chimio-mécanique aqueux pour décolorer et régénérer des polyoléfines mixtes
Une nouvelle approche permet de traiter des plastiques polyoléfiniques hétérogènes par un procédé chimio-mécanique en milieu aqueux, destiné à contourner les limites du recyclage strictement mécanique (dégradation irréversible des chaînes, odorisation, mélange imparfait) sans basculer vers une dépolymérisation coûteuse. Le principe repose sur l’utilisation d’eau portée au-delà de son point d’ébullition sous pression, créant un environnement physico-chimique où les polymères passent transitoirement dans un état favorable à l’interdiffusion et au mélange à l’échelle micrométrique, tout en facilitant l’extraction d’impuretés. Le traitement est décrit comme capable d’éliminer des composés organiques volatils associés à l’odeur de recyclé, et de désorber des pigments afin de rapprocher la teinte du matériau régénéré de celle d’une résine vierge. Point critique, la cinétique d’exposition thermique est finement pilotée : en limitant la durée de séjour, le procédé réduit la scission de chaînes et préserve la masse molaire, condition clé pour restaurer rigidité, ténacité et aptitude à la transformation lors d’une remise en œuvre ultérieure. Par sa sobriété énergétique relative et sa capacité à purifier des flux mélangés et colorés, cette voie ouvre des perspectives de recyclats de qualité comparable aux grades neufs, compatibles avec une montée en échelle industrielle et une réduction tangible des mises en décharge ou de l’incinération.
https://phys.org/news/2026-01-chemi-mechanical-pigments-properties-recycled.html
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Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
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Les partenaires
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Waters_logo_stacked_K_web-NEW
http://www.waters.com
ICS
https://www-ics.u-strasbg.fr/
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cnrs
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lrccp
http://www.ispa.asso.fr
Logo-ChemSuD
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http://www.hutchinson.com/fr
arkema
http://www.coatex.com
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