Le réseau
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L'organisation
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La structure de veille et de réflexion prospective
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Actualités
Des polyesters circulaires obtenus par copolymérisation directe du CO2
Une copolymérisation alternée du dioxyde de carbone avec des bicyclobutanes ou des bicyclopentanes permet d’obtenir des polyesters de masse molaire élevée contenant jusqu’à 50 % molaire de CO2. Un catalyseur organique simple initie la réaction et produit des chaînes dont les cycles intégrés au squelette ajustent les propriétés thermiques et mécaniques. Les polyesters issus des bicyclobutanes résistent à l’hydrolyse sur une large plage de pH mais peuvent être dépolymérisés sélectivement pour régénérer plus de 90 % du monomère. Des cycles successifs de dépolymérisation et de repolymérisation confirment la possibilité d’une boucle chimique fermée.
Nature Une plateforme microbienne pour produire les monomères de plastiques chimiquement recyclables
Des polykétide synthases hybrides ont été conçues pour produire, dans des bactéries, différents β-céto-δ-lactones utilisables comme précurseurs de polydikétoénamines recyclables. Le criblage informatique de 144 structures a permis de relier la solvatation des monomères à la température nécessaire pour déconstruire les polymères. Les structures testées présentent des températures de transition vitreuse comprises entre 53 et 98 °C ainsi que des températures de dépolymérisation modulables entre 0 et 60 °C. Les polymères caractérisés ont encore été préparés à partir de monomères synthétisés chimiquement, mais la production biologique proche de 2 g/L démontre la faisabilité d’une future plateforme fermentaire alimentée par des ressources renouvelables.
L’IEM et l’ICGM développent des nanoparticules de polyélectrolytes partiellement biosourcés en milieu aqueux
Des chercheurs de l’Institut européen des membranes et de l’Institut Charles Gerhardt Montpellier, associés à l’Université de Montpellier, au CNRS et à l’ENSCM, ont étudié l’auto-assemblage aqueux de poly(acides amiques) partiellement biosourcés avec une polyéthylèneimine ramifiée. Les précurseurs macromoléculaires sont issus de diamines à base de difurfurylamine puis convertis en sels solubles dans l’eau afin d’éviter le recours aux solvants organiques habituellement employés pour ces polymères. Selon la structure du squelette et le rapport de charges, les mélanges conduisent à des nanoparticules stables de 10 à 20 nm ou à des agrégats de complexes polyélectrolytiques plus denses. Le travail, soutenu par le projet ANR POMENVI, met en évidence le rôle déterminant de l’accessibilité des charges et valorise les compétences montpelliéraines en polymères biosourcés, membranes et auto-assemblage colloïdal.
SpringerLink Comparaison économique des principales voies de recyclage des plastiques
Une analyse technico-économique compare le recyclage mécanique, la dissolution sélective, la glycolyse, la méthanolyse et l’hydrolyse enzymatique du PET, du polyéthylène et du polypropylène. Dans les hypothèses retenues, le recyclage mécanique demeure la solution la moins coûteuse, tandis que les procédés par solvant ou par enzymes produisent des matières plus pures au prix d’investissements et de coûts opératoires supérieurs. Parmi les voies chimiques évaluées, la glycolyse présente la meilleure compétitivité économique. Le rendement matière, le prix des balles de déchets et la capacité de l’installation apparaissent comme les variables les plus influentes.
SpringerLink L’IPREM développe des latex aqueux biosourcés à partir d’un acrylate terpénique et d’une huile naturelle
Une collaboration impliquant Laurent Billon, professeur à l’Université de Pau et des Pays de l’Adour et chercheur à l’IPREM, UMR CNRS 5254, propose une voie de polymérisation aqueuse combinant un monomère acrylique d’origine terpénique et un tensioactif naturel extrait de graines d’Opuntia ficus-indica. Les procédés d’émulsion permettent de préparer des latex de polystyrène, de poly(acrylate de menthyle) et de leurs copolymères sous forme de particules sphériques de l’ordre de 70 à 200 nm. Les formulations optimisées atteignent des conversions allant jusqu’à 79 % sans coagulation et présentent une stabilité colloïdale prolongée. Ces travaux mettent en avant les compétences françaises de l’IPREM en polymérisation en milieu dispersé, colloïdes et matériaux macromoléculaires issus de ressources renouvelables.
Microsphères creuses en polyacrylate pour le refroidissement radiatif
Des microsphères creuses dotées d’une coque en poly(triméthylolpropane triacrylate) sont préparées avec un cœur volatil éliminé après polymérisation. Leur diamètre moyen est proche de 2 µm pour une paroi d’environ 50 nm. Incorporées dans un revêtement textile, elles combinent une réflectance solaire supérieure à 80 % et une émissivité infrarouge dépassant 90 %. Les essais en extérieur montrent un écart maximal de température de surface de 6,9 °C et une diminution de plusieurs degrés de la température au contact de la peau.
SpringerLink Lorem ipsum dolor sit amet, consectetur adipiscing elit. Sed posuere tincidunt quam sit amet viverra. Nam in consequat nulla. Nunc rhoncus orci vitae arcu sagittis, in auctor nibh posuere. Donec ut nulla id enim tempor feugiat.
Adhérez au GFP
Devenez un membre et découvrez les avantages d’un abonnement GFP.
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Sections locales GFP
Lorem ipsum dolor sit amet, consectetur adipiscing elit. Etiam feugiat quis risus quis tempus. Morbi pharetra volutpat ligula ut placerat. Morbi sagittis ornare tellus, at molestie urna suscipit id. Praesent non est quis ante pretium ullamcorper. Lorem ipsum dolor sit amet, consectetur adipiscing elit. Vestibulum ante ipsum primis in faucibus orci luctus et ultrices posuere cubilia Curae; Integer sodales nisi justo, a varius nisi viverra accumsan. Quisque eleifend velit sed suscipit convallis. Donec ac facilisis massa. Donec euismod erat molestie nisi condimentum mattis. Nunc eu eros lacinia, vestibulum nibh vitae, varius magna. Aliquam erat volutpat. Suspendisse potenti.
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Les partenaires
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LPMC
http://www.ispa.asso.fr
logo-ispa_coul_fond-fonce
http://www.ispa.asso.fr
hutchinson
http://www.hutchinson.com/fr
cnrs
http://www.ispa.asso.fr
Waters_logo_stacked_K_web-NEW
http://www.waters.com
arkema
http://www.coatex.com
Logo-ChemSuD
http://www.ispa.asso.fr
ICS
https://www-ics.u-strasbg.fr/
lrccp
http://www.ispa.asso.fr
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